Theory of D-(-)-Luciferin and Dehydroluciferin in Acidic or Basic Solution
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概要
- 論文の詳細を見る
In order to understand the molecular mechanism of firefly' bioluminescence, theobserved absorption spectra of o-( -)-luciferin (LH.) and dehydroluciferin (L) inacidic or basic solution are reproduced by the LCAO-ASMO-SCF-Cl calculation onm-electrons.It is thus found that the first absorption band of LH. in basic solution is ascribableto the intramolecular charge-transfer from benzotlniazole to thiazoline ring, and thatthis absorption band is considerably affected by the reaction field due to solventmedium. On this basis, we cliscuss the formation process of the excited state ofoxyluciferin (oxy-L) caused by the oxidation of L14., together' with CREEL (Chemi-cally Initiated Electron Exchange Luminescence) mechanisms proposed by several in-vestigators.
- 社団法人日本物理学会の論文
- 1985-12-15
著者
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Suzuki Hideo
Department of Information and Network Science, Chiba Institute of Technology
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和田 信雄
Graduate School Of Arts And Sciences University Of Tokyo
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HONDA Makoto
Department of Physics, Faculty of Science, Naruto University of Education
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Wada Naohisa
Department Of Physics Of General Education School Of Engineering Toyo University
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Wada Naohisa
Department Of General Education Of Physics School Of Engineering Toyo University
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Wada Naohisa
Department Of Applied Chemistry And Biotechnology Graduate School Of Engineering University Of Fukui
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Honda Makoto
Department Of Physics Faculty Of Science Naruto University Of Education
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Wada N
Yamagata Univ. Yamagata Jpn
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Wada N
Univ. Tokyo Tokyo
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Honda M
Max Planck Inst. Quantum Optics Garching Deu
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Wada Nobuo
Department Of Physics College Of Arts And Science University Of Tokyo
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HONDA Mitsuo
Department of General Education of Physics,School of Engineering,Toyo University
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Honda M
Department Of Physics Faculty Of Science Naruto University Of Education
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Suzuki Hideo
Department Of Cardiology Surugadai Nihon University Hospital
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Suzuki Hideo
Department of Bioscience Research, Tsukuba Research Laboratory, Toagosei Co., Ltd.
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