Indirect Spin-Spin Coupling in InP Investigated by Triple-Resonance NMR under Magic-Angle Spinning (Condensed Matter : Electronic Structure, Electrical, Magnetic and Optical Properties)
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概要
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The ^<31>PNMR spectra were measured using ^<31>P, ^<113>In and ^<115>In triple-resonance and magic-angle spinning (MAS) to investigate an indirect spin-spin interaction in undoped and Fe-doped InP semiconductors. The linewidth of the static NMR spectrum obtained by cross polarization (CP) of ^<115>In → ^<31>P with ^<115>In decoupling was explained by the lattice sum of ^<31>P-^<31>P dipolar couplings. On the other hand, the linewidth of the MAS NMR spectrum obtained by CP of ^<115>In → ^<31>P without ^<115>In decoupling was interpreted by the isotropic indirect interaction of neighboring ^<115>In-^<31>P spins. We obtained 10 equally spaced lines corresponding to ^<113>In spin state from the MAS NMR spectrum measured with CP from rare ^<113>In to ^<31>P under ^<115>In decoupling. From these experiments, the isotropic contributions of the electron-mediated nuclear coupling between the nearest neighboring ^<113,115>In-^<31>P spins was obtained as |^1J^<iso>(I,S)| = 224 ± 5 Hz for undoped and Fe-doped InP samples. The ^1J^<iso>(I,S) value was found to be unaffected by the carrier with the density in the range of 10^7-10^<15> cm^<-3>.
- 社団法人日本物理学会の論文
- 2004-04-15
著者
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Shimizu T
National Institute For Materials Science
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SHIMIZU Tadashi
National Research Institute for Metals
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HASHI Kenjiro
National Institute for Materials Science (NIMS)
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GOTO Atsushi
National Institute for Materials Science
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OHKI Shinobu
National Institute for Materials Science
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IIJIMA Takahiro
National Institute for Materials Science
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OHKI Shinobu
CREST, Japan Science and Technology Agency
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SHIMIZU Tadashi
Institute for Solid State Physics,University of Tokyo
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Iijima Takahiro
National Institute For Materials Science:(present Address)department Of Chemistry Graduate School Of
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Shimizu Tadashi
National Inst. For Materials Sci.
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Shimizu Tadashi
Advanced Nano Characterization Center National Institute For Materials Science
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Shimizu T
National Inst. Materials Sci. Ibaraki Jpn
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Shibuya T
Univ. Tokyo Tokyo Jpn
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Goto Atsushi
National Research Institute For Metals
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Goto Atsushi
Institute For Solid State Physics University Of Tokyo
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Shimizu T
National Research Laboratory For Metal
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Shimizu Tadashi
High-field Nmr Group Advanced Nano Characterization Center
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Shimizu Tadashi
Issp Of The Univercity Of Tokyo
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Goto A
National Research Laboratory For Metal
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Hashi K
National Institute For Materials Science
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Hashi Kenjiro
National Institute For Materials Science
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Shimizu Tadashi
National Institute For Material Sciences
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Shimizu Tadashi
National Institute For Material Science
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Goto Atsushi
National Institute for Materials Science (NIMS)
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