Structure and Electronic Properties of Amorphous Ge-Pd Alloys Manifesting the Metal-Insulator Transition. : II.Photoemission Spectroscopy and Electronic Structure Calculations
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概要
- 論文の詳細を見る
Photoetnission valence band spectrat of' autuorphous Ge -Pd ;xlloys prodtrced by Ar-ion-bearaasptrttering are raueastrred with XPS and UPS techraiqtres over a xvide r'atage of Pd concentration.A Pd-derived band coraaj.cosed of' Pd47-Ge4p botudizag states develops xvitla Pd concentration srndgovertas the tupper valence band region ira laigh cot?ccentrations. The UPS profile at the Ferraaiedge shoxvs that a unetallic conti?attotus band is ['ortaued in alloys above 1,3% Pd. To iraterpretthe plaotoemission spectra anad rexzeal tlte electronic strtucttrre of tlaese anaorphotts alloys, DV-X(lnaolecttlar orbital calctrlations are perfortned for Gej7 ,.Pd. (n : O, 1, 2, 4, 5) cltrsters xvitltdiamond strtrcttrre wltich naay sitntrlate sorne local strtrcttrres of' ataaorphotrs atlloys of' IOXV Pdconcentrations. Calcttlated partial and total density of states well repr'odtrce the valence lcandfeattrres revearled by XPS ?xnd UPS. A bandstrtrcture claange frouaa an open barad to a contitatrotrsband at tlue Fernai level caused by alloying with Pd is 21180 corafir'tned 1.cy the calcttlation. Thelocalization-delocalization behavior of tlae rauo1ecul?rr orbital at the Fernni level ita the cltrsterappears to be related xvitla tl'ae metal-instrlator transition in 21l1l0FPl1OUS Ge-Pd 21llOVS.
- 社団法人日本物理学会の論文
- 1999-11-15
著者
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SUZUKI Atsuko
Department of Geriatric Medicine, Osaka University Graduate School of Medicine
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Tanaka K
Institute Of Earth And Space Science Graduate School Of Science Osaka University
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田中 宏治
Med.safe.res.labs. Sankyo Co. Ltd. Of Shizuoka Pref.
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Suzuki A
Nagoya Inst. Technol. Nagoya
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Tanaka K
Department Of Toxicology Graduate School Of Pharmaceutical Sciences Osaka University:(present Office
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ENDO ATSUSHI
Department of Applied Chemistry, Faculty of Engineering, Utsunomiya University
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Endo Atsushi
Department Of Materials Science And Engineering Nagoya Institute Of Technology
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TANAKA Kazuhide
Department of Metallurgy, Nagoya Institute of Technology
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Tanaka Katsushi
Department Of Materials Science And Engineering Graduate School Of Engineering Kyoto University
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Tanaka Keiichi
Dep. Toxicol. Grad. School Pharmaceut. Sci. Osaka Univ.
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Tanaka K
Department Of Physics Graduate School Of Science Kyoto University
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Tanaka K
Kumamoto Univ. Kumamoto Jpn
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Kojitani Takatoshi
Res. Inst. Of Pharmaceutical Sciences Musashino Univ.
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Tanaka Kazuhide
Department Metallurgical Engineering Nagoya Institute Of Technology
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Suzuki A
Tezukayama Coll. Nara Jpn
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Tanaka K
Kobe‐gakuin Univ. Kobe Jpn
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Suzuki Atsuko
Department Of Cardiology Seirei Mikatahara Hospital
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