Balanced Ambipolar Transport of the Composite Film of a Carbazole--Benzothiadiazole Copolymer with a Fullerene Derivative
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概要
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The ambipolar field-effect transport of a narrow-bandgap copolymer poly[N-9''-heptadecanyl-2,7-carbazole-alt-5,5-(4',7'-di-2-thienyl-2',1',3'-benzothiadiazole)] (PCDTBT) mixed with a fullerene derivative [6,6]-phenyl-C<inf>61</inf>-butyric methyl ester (PCBM) is observed in the PCBM weight ratio of 50--90 wt %. The hole mobility decreases with increasing PCBM content by only less than one order of magnitude, indicating that the PCDTBT structure is not much perturbed by PCBM. This is supported by the absence of a blue shift of the polymer absorption band when PCBM is loaded. Balanced hole and electron transport was achieved at {\sim}80 wt %, in good agreement with the ratio of the highest conversion efficiency of the solar cell.
- 2013-05-25
著者
-
Kuroda Shin-ichi
Department Of Applied Physics Nagoya University
-
Ito Hiroshi
Department Neurosurgery Tokyo Medical College
-
Watanabe Shun-ichiro
Department Of Applied Physics Nagoya University
-
Iwata Takanori
Department of Applied Physics, Nagoya University, Nagoya 464-8603, Japan
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