The electrical properties of La2-xSrxNiO4 (0.LEQ.x.LEQ.1).
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概要
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The electrical resistivities and Seebeck coefficients of mixed oxides, La<SUB>2−<I>x</I></SUB>Sr<I><SUB>x</SUB></I>NiO<SUB>4</SUB>, have been determined under an He atmosphere at 77.4–673.2 K. It has been shown that the temperature dependences of the Seebeck coefficients of the oxides were fairly well approximated by this equation: <I>S</I>=<I>AT</I>+<I>B</I>+<I>C</I>⁄<I>T</I>, where <I>T</I> is the thermodynamic temperature. The coefficients of the equation, <I>A</I>, <I>B</I>, and <I>C</I>, were given by the least-squares method. The metal-semiconductor ratios {α≡(<I>C</I>⁄<I>T</I>)⁄(<I>AT</I>+<I>C</I>⁄<I>T</I>)} were given to characterize the thermoelectrical properties of La<SUB>2−<I>x</I></SUB>Sr<I><SUB>x</SUB></I>NiO<SUB>4</SUB>. The maximal activation energies (<I>E</I><SUB>a</SUB>(resis.) and <I>E</I><SUB>a</SUB>(Seebeck)) and the maximal metal-semiconductor ratio (α) were obtained with the strontium concentration of La<SUB>2−<I>x</I></SUB>Sr<I><SUB>x</SUB></I>NiO<SUB>4</SUB> at <I>x</I>=0.5. The lattice distortion of the oxides is responsible for the maxima of the activation energies and of the metal-semiconductor ratio at <I>x</I>=0.5.
- 公益社団法人 日本化学会の論文
著者
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Kondo Shin-ichi
Department Of Applied Physics Faculty Of Engineering Fukui University
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Takayama Shin-ichi
Department Of Cardiology And Nephrology Shizuoka Central Prefectural Hospital
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Suzuki Yuichi
Department Of Bioscience And Chemistry Faculty Of Agriculture Hokkaido University
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Suzuki Yasuo
Department Of Applied Physics Faculty Of Engineering Fukui University
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Ishikawa Kenji
Department of Earth and Space Science, Graduate School of Science, Osaka University, 1-1 Machikaneyama, Toyonaka, Osaka 560-0043, Japan
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Suzuki Yuichi
Department of Industrial Chemistry, Faculty of Engineering, Meiji University
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Shimada Kazuhiko
Department of Chemical Engineering, Faculty of Engineering, Doshisha University
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Shimada Kazuhiko
Department of Industrial Chemistry, Faculty of Engineering, Meiji University
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