Resonant Inverse Photoemission and Many-Body Effect in Nickel
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概要
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We calculate a resonant inverse photoemission spectroscopy (IPES) spectrum at the Ni 3pcore threshold (3d" -f 3p'3d"" -f 3d"'), f'roun a viewpoint of a tnany-body configurationinteraction (Cl), on the basis of the Anderson impurity naodel. The calctrlated IPES spectrurnexhibits a single tnain peak .just above the Fermi level Ev tunder off-resonance, while it hasa shoulder extending to 4 eV above Ev under on-resonance conditions. Under on-resonanceconditions, the main peak intensity shows a dip whose tnagnitude is a function of the incidentelectron energy e, while the shotulder is resonantly enhanced. The interference between thedirect 3d' + 3d' and resonant 3d' + 3p'3d" + 3d' processes and Cl in both the initial andfinal states leads to the above restult. Resonant IPES is therefore considered to be a promisingrnethod of directly deternaining whether a 3d' configuration in the initial state, inferred byanalysis of variotrs high-energy spectroscopic data, does in fact exist. The main peak is assignedto the bonding state of 3d" and 3d' configtrratioras and the shoulder a non-bonding and theanti-bonding states of them.
- 社団法人日本物理学会の論文
- 1997-06-15
著者
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JO Takeo
Department of Quantum Matter,ADSM,Hiroshima University
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Tanaka A
Adsm Hiroshima University
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Tanaka Arata
Department Of Quantum Matter Adsm Hiroshima University
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Tanaka Arata
Department Of Materials Science Faculty Of Science Hiroshima University
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Jo T
Department Of Quantum Matter Adsm Hiroshima University
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Jo Takeo
Department Of Materials Science Faculty Of Science Hiroshima University
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