ESR Studies on 3d Transition Metal Intercalation into Lavered TiS_2 Crystals
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概要
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Extensive X-band ESR measurements have been made on the 3d transitionmetal intercalation compound M.TiS. (M=V, Cr, Mn, Fe, Co, Ni; 0<,X'<1)over the temperature range 300-77 K. The variations of the intra- and interlayerspacings with intercalation of guest atoms are presented. Fe and xi intercalatesdo not show an>' ESR sisnals. Masnetic interactions are ineffective in V.TiS.,while in Cr,TiS. and Mn.TiSz dipolar interactions are dominant and theseparamagnetic atoms undergo a thermally activated motion in the interlayers.Co.TiS. becomes ferromagnetic below T. (<140K) and their temperaturedependence of Iinewidth is very similar to those in itinerant ferromagnets likeCoS., suggesting the formation of a low spin state near the host Ti d-band. Theanisotropies in the y-value and linewidth are notable in these layered intercalates.
- 社団法人日本物理学会の論文
- 1985-01-15
著者
-
Inoue Masasi
Department Of Applied Physics Fukui University
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Negishi Hiroshi
Department Of Materials Science Faculty Of Science Hiroshima University
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