A novel formation of phenyl-substituted pyridines by the reaction of N-(diphenylphosphinyl)-1-azaallyl anions with .ALPHA.,.BETA.-unsaturated carbonyl compounds. A new synthetic equivalent of primary vinylamines.
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概要
- 論文の詳細を見る
The <I>N</I>-phosphinyl-1-azaallyl anions, which were derived from the corresponding imine or enamine, reacted with α,β-unsaturated carbonyl compounds to afford phenyl-substituted pyridines along with 1-propanone and 1,5-pentanedione derivatives. A plausible mechanism involving a sequence of Michael addition and intramolecular aza-Horner-Wittig reaction is described, and the 1-azaallyl anions were found to behave as a synthetic equivalent of primary vinylamines.
- 公益社団法人 日本化学会の論文
著者
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Kato Hiroshi
Department Of Applied Biological Chemistry Graduate School Of Agricultural And Life Sciences The Uni
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Kobayashi Tomoshige
Department Of Chemistry Faculty Of Science Shinshu University
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Kakiuchi Hidetaka
Department of Chemistry, Faculty of Science, Shinshu University
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Kawate Hiroshi
Department of Chemistry, Faculty of Science, Shinshu University
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