Infrared Band Shape of the C–I Stretching Vibration of Methyl Iodide in Solutions

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概要

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• The infrared band shapes of the fundamental and overtone C–I stretching vibrations of methyl iodide in solutions are well approximated by the superposition of Lorentzian functions. From a comparison of the bandwidths of the ν<SUB>3</SUB>(→1), ν<SUB>3</SUB>(1→2), and ν<SUB>3</SUB>(0→2) transitions, it is pointed out that the vibrational relaxation of the translational-diffusion type proposed by Bratos <I>et al.</I> contributes to the band-widths, in addition to reorientational relaxation. A slight deviation from the Lorentzian function was observed in the low-frequency region of the fundamental band.

• 公益社団法人 日本化学会の論文

著者

• Kimura Masao

  Department of Chemistry Nagoya University

• Fujiwara Kenji

  Department of Chemistry, Faculty of Science, Hokkaido University

• Fukushi Kohji

  Department of Chemistry, Faculty of Science, Hokkaido University

• Ikawa Shun-ichi

  Department of Chemistry, Faculty of Science, Hokkaido University

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