Unconventional Superconductivity and Nearly Ferromagnetic Spin Fluctuations in Na_xCoO_2・_yH_2O(Condensed Matter : Electronic Structure, Electrical, Magnetic and Optical Properties)

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Co nuclear-quadrupole-resonance (NQR) studies were performed in the recently discovered superconductor Na_xCoO_a-_yH_2O to investigate physical properties in the superconducting (SC) and normal states. Two samples from the same Na_xCoO_2 were examined, a SC bilayer-hydrate sample with T_c 〜 4.7 K and a non-SC monolayer-hydrate sample. From the measurement of nuclear-spin lattice relaxation rate 1/T_1 in the SC sample, it was found that the coherence peak is absent just below T_c and that 1/T_1 is proportional to temperature far below T_c. These results, which are in qualitative agreement with the previous result by Fujimoto et al., suggest strongly that unconventional superconductivity is realized in this compound. In the normal state, l/T_1T of the SC sample shows a gradual increase below 100 K down to T_c, whereas 1/T_1T of the non-SC sample shows the Korringa behavior in this temperature range. From the comparison between 1/T_1T and χ_<bulk> in the SC sample, the increase in 1/T_1T is attributed to nearly ferromagnetic fluctuations. These remarkable findings suggest that the SC sample possesses nearly ferromagnetic fluctuations, which are possibly related to the unconventional superconductivity in this compound. The implication of this finding is discussed.
社団法人日本物理学会の論文
2003-12-15