Evidence for the similarity recognition hypothesis. Structure dependence of the selectivity in oxidation of a pair of associating thiols each having an alkyl group.

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概要

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• In base-catalyzed oxidation of a pair of associating thiols [HSCH<SUB>2</SUB>–CONHCONH–R<SUP>1</SUP> and HSCH<SUB>2</SUB>CH<SUB>2</SUB>–NHCONHCO–R<SUP>2</SUP>] (R<SUP>1</SUP>=<I>n</I>-C<SUB>4</SUB>H<SUB>9</SUB>, R<SUP>2</SUP>=<I>n</I>-C<I><SUB>n</SUB></I>H<SUB>2<I>n</I>+1</SUB>) with oxygen, the selectivity (a measure of molecular recognition) at 35.0°C reached a maximum for R<SUP>1</SUP>=R<SUP>2</SUP> (=<I>n</I>-C<SUB>4</SUB>H<SUB>9</SUB>) both in aqueous acetonitrile (<I>n</I>=2 to 6) and in aqueous ethanol (<I>n</I>=3 to 5).

• 公益社団法人 日本化学会の論文

著者

• Isago Takashi

  Department Of Chemistry College Of Science And Engineering Aoyama Gakuin University

• Endo Tadashi

  Department Of Applied Chemistry Faculty Of Engineering Tohoku University

• Kato Jun-ichi

  Department of Applied Chemistry, Faculty of Science and Engineering, Kinki University

• Ueda Takeshi

  Department Of Energy Engineering And Science Nagoya University

• Ito Masato

  Department Of Applied Chemistry Graduate School Of Science And Engineering Tokyo Institute Of Techno

• Suzuki Takashi

  Department Of Anatomic Pathology Tohoku University School Of Medicine

• Misaka Makoto

  Department of Chemistry, College of Science and Engineering, Aoyama Gakuin University

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