Interdiffusion of zinc ions in aluminium Cobalt(II) oxide and aluminium nickel(II) oxide.
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概要
- 論文の詳細を見る
The interdiffusion coefficients \tilde<I>D</I> of Zn<SUP>2+</SUP> ions in aluminium cobalt(II) oxide (cobalt aluminate) and aluminium nickel(II) oxide (nickel aluminate) were measured. In the former \tilde<I>D</I> is independent of the concentration of the composition-dependent cation vacancies, while in the latter it decreases with increase in the concentration of cation vacancies. The difference in the distribution of cations and cation vacancies in the spinel lattice has a great effect on the interdiffusion coefficients of Zn<SUP>2+</SUP> ions. The results were interpreted by means of the vacancy mechanism for Co<SUP>2+</SUP> and Ni<SUP>2+</SUP> ions and the interstitial or interstitialcy mechanism for Zn<SUP>2+</SUP> ions. The activation energy is independent of the concentration of Zn<SUP>2+</SUP> ions or cation vacancies; 355 kJ mol<SUP>−1</SUP> for cobalt aluminate and 364 kJ mol<SUP>−1</SUP> for nickel aluminate.
- 公益社団法人 日本化学会の論文
著者
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Matsubara Takao
Department Of Cardiology Ishikawa Prefectural Central Hospital
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Takata Masasuke
Department Of Electrical Engineering Nagaoka University Of Technology
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Koumoto Kunihito
Department Of Applied Chemistry Graduate School Of Engineering Nagoya University
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Yanagida Hiroaki
Department Of Applied Chemistry Faculty Of Engineering University Of Tokyo
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KOUMOTO Kunihito
Department of Industrial Chemistry, Faculty of Engineering, The University of Tokyo
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Matsubara Takao
Department of Industrial Chemistry, Faculty of Engineering, The University of Tokyo
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