Effect of Solute Adsorption Properties on Its Separation from Supercritical Carbon Dioxide with a Thin Porous Silica Membrane
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概要
- 論文の詳細を見る
A thin porous silica membrane (average pore size of 3.3 mm) was prepared by the sol-gel method and used to separate the solute from supercritical carbon dioxide. The characteristics of solute permeation were investigated in respect of the adsorption properties of the solute, the desorption rate of the solute from the membrane being measured and the potential energy of solute near the silica surface being calculated by the molecular modeling technique. It was found that caffeine was strongly adsorbed to the surface and then slowly desorbed to form an adsorption layer, making the pores narrower and causing a molecular-sieving effect. Therefore, the rejection value was positive. On the other hand, the rejection value of n-octanoic acid, which was well adsorbed and rapidly desorbed, was negative. It is presumed that the molecules filled the pores due to their potential energy and were then forced to flow through the pores by the transmembrane pressure.
- 社団法人日本農芸化学会の論文
- 1996-12-23
著者
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NAKAMURA KOZO
Department of Orthopaedic Surgery, Faculty of Medicine, The University of Tokyo
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Fujii T
Kyoto Univ. Kyoto
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中村 薫
京大 化研
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中村 厚三
Univ. Tokyo Tokyo Jpn
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Fujii T
Department Of Applied Biological Chemistry The University Of Tokyo
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Fujii Tomoyuki
Department Of Food Science And Technology Niigata University Of Pharmacy And Applied Life Sciences
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TOKUNAGA Yoshihiro
Department of Applied Biological Chemistry, The University of Tokyo
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Tanaka Y
Kyushu Univ. Fukuoka Jpn
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Nagahama Kazuhiro
Department Of Applied Microbial Technology The Kumanoto Institute Of Technology
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Fujii T
Inst. Biol. Sci. Univ. Tsukuba
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Fujii Tomoyuki
Department Of Applied Biological Chemistry The University Of Tokyo
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Fujii T
Div. Of Bioresource Sci. Graduate School Of Horticulture Chiba Univ.
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Nakamura Kozo
Department Of Bioscience And Biotechnology Faculty Of Agriculture Shinshu University
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Nakamura Kahoru
Department Of Nutrition Tokyo University Of Agriculture
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Tokunaga Yoshihiro
Laboratory Of Food Chemistry Division Of Applied Biological Chemistry Department Of Bioscience And B
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Nakamura Kozo
Department Of Agricultural Chemistry The University Of Tokyo
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Tokunaga Yoshihiro
Department Of Applied Biological Chemistry The University Of Tokyo
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