Magnetic Phase Transition of Ni(NH_3)_2Ni(CN)_4・2C_<12>H_<10>
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概要
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The magnetic susceptibility and the specific heat of Ni(NH_3)_2Ni(CN_4)・2C_<12>H_<10> have been measured between 0.35 K and 20 K on a powder specimen. The crystalline-field splitting energy of the Ni^<++> -ion spin triplet is estimated to be 2.5±0.3 K with doublet ground state (S_z=±1). Together with a layer structure of the magnetic ions in this clathrate compound, the magnetic spins can be regarded as forming a two-dimensional Ising-like system. A symmetric logarithmic divergence of the specific heat is actually observed at T_N=0.800±0.005K.
- 社団法人日本物理学会の論文
- 1976-12-15
著者
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Watanabe Takashi
Department of Chemistry, Graduate School of Science, Kyoto University
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SIMIZU Satoru
Department of Neurosurgery, Kitasato University School of Medicine
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NISHITANI Tomio
Department of Physics, Faculty of Science, Hokkaido University
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Watanabe Takashi
Department Of Cardiothoracic Surgery Nagoya University School Of Medicine
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Nishitani Tomio
Department Of Physics Faculty Of Science Hokkaido University:(present Address) Osaka Oxygen Industries Ltd.
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Watanabe Takashi
Department Of Physics Faculty Of Science Hokkaido University
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Watanabe Takashi
Department Of Applied Physics Tohoku University
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