Magnetic Properties of Ni(CN)_2・NH_3・C_6H_6
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概要
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Ni^<++> ions of Ni(CN)_2・NH_3・C_6H_6 are linked up making the two dimensional square network through the -C-N- bonds. Magnetic susceptibility, magnetization, nuclear magnetic resonance of this complex compound were measured at liquid helium and liquid hydrogen temperature ranges. From the present result, the magnetic moment is 2.18 μ_B and θ=-2.7°K in the expression x=C/(T-θ). The result of saturation magnetization shows the fact that one half of Ni^<++> ions in this compound is in the paramagnetic state (S=1) with ∼3.0 μ_B and the other half in the diamagnetic one (S=0) with the zero magnetic moment. This compound is antiferromagnet that has a magnetic phase transition at T_N=2.37±0.01°K which agrees with the inflection point on the susceptibility versus temperature curve at zero external field. In the antiferromagnetic state, the value of anisotropy field was found at H_A≈8kOe.
- 社団法人日本物理学会の論文
- 1968-08-05
著者
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Watanabe Takashi
Department of Chemistry, Graduate School of Science, Kyoto University
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MARUYAMAUCHI Tsuyoshi
Department of Physics, Faculty of Science Hokkaido University
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Maruyamauchi Tsuyoshi
Department Of Physics Faculty Of Science Hokkaido University
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Takayanagi Sigeru
Department Of Physics Faculty Of Science Hokkaido University
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Watanabe Takashi
Department Of Cardiothoracic Surgery Nagoya University School Of Medicine
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Watanabe Takashi
Department Of Applied Physics Tohoku University
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