Mechanism of resonant two-photon transitions via repulsive intermediate states. Experimental and theoretical studies on I2 vapor.
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概要
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Mechanisms of resonant two-photon transitions <I>via</I> repulsive intermediate states are experimentally and theoretically studied. Polarization ratios, <I>Ω</I>=σ<SUB>∞</SUB>⁄σ<SUB>↑↑</SUB> (where σ<SUB>∞</SUB> and σ<SUB>↑↑</SUB> are the cross section of the two-photon transitions obtained by the circularly polarized light and that by the linearly polarized light, respectively) of the two-photon excitation of iodine vapor have been measured in the wavelength range of 420–510 nm. An expression for the polarization ratio for the two-photon absorption in which both simultaneous and sequential processes take place has been presented. The polarization ratios calculated by using the δ-function approximation for the repulsive intermediate states as a function of the laser frequency for the iodine molecule system explain qualitatively the experimental result. This indicates that both the simultaneous and the sequential process take place in the frequency region measured.
- 公益社団法人 日本化学会の論文
著者
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Shiraishi Jun
Department Of Cardiology Kyoto First Red Cross Hospital
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Fujimura Yuichi
Department Of Chemistry Graduate School Of Science Tohoku University
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Kawasaki Masahiro
Chemistry Department Of Resources Faculty Of Engineering Mi'e University
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Sato Hiroyasu
Chemistry Department Of Resources Faculty Of Engineering Mi'e University
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Nakajima Takeshi
Department of Chemistry Faculty of Science Tohoku University
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Kasatani Kazuo
Chemistry Department of Resources, Faculty of Engineering, Mi'e University, Tsu 514
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Tanaka Ikuzo
Department of Chemistry, Tokyo Institute of Technology
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Kasatani Kazuo
Chemistry Department of Resources, Faculty of Engineering, Mi'e University
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