Ultrafast Photoconversion from Charge Density Wave State to Mott-Hubbard State in One-Dimensional Extended Peierls-Hubbard System of Br-Bridged Pd Compound(Condensed matter: electronic structure and electrical, magnetic, and optical properties)

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概要

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• Photoconversion from a charge density wave (CDW) state to a Mott-Hubbard (MH) state in a one-dimensional (1D) extended Peierls-Hubbard system is observed by femtosecond (fs) reflection spectroscopy. The Br-bridged Pd compound examined is located near the CDW-MH phase boundary, and the irradiation of a fs laser pulse causes the instantaneous formation of a 1D MH domain without alternation of bridging-Br displacements. This result demonstrates the important role of intersite Coulomb repulsion in the transition, and in the stabilization of the CDW state. The formation of the MH domain is followed by a coherent oscillation with a period of 360fs attributable to the relaxation of the bridging-Br displacements coupled with the charge-transfer between neighboring Pd ions.

• 社団法人日本物理学会の論文
• 2006-12-15

著者

• Okamoto Hiroshi

  Department Of Cardiovascular Medicine Hokkaido University Hospital

• Yamashita Masahiro

  Department Of Bioengineering Tokyo Institute Of Technology

• MATSUZAKI HIROYUKI

  Department of Nuclear Engineering and Management, School of Engineering, The University of Tokyo, To

• 山下 護

  徳島工短

• 山下 護

  Department Of Physics Engineering Faculty Of Engineering Mie University

• Yamashita Makoto

  Department Of Applied Physics Osaka University

• Miyasaka Hitoshi

  Kansai Electric Power Co. Technical Research Center Environmental Research Center:rite Amagasakti 2n

• Matsuzaki Hiroyuki

  Department Of Advanced Materials Science Graduate School Of Frontier Sciences University Of Tokyo

• Yanagimoyo Masanobu

  Department Of Chemistry Faculty Of Science Ehime University

• Miyasaka Hitoshi

  Department Of Chemistry Faculty Of Science Tokyo Metropolitan University

• Okamoto Hiroshi

  Institute For Materials Research Tohoku University

• Yamashita Masahiro

  Department Of Chemistry Graduate School Of Science Tokyo Metropolitan University

• Okamoto Hiroshi

  Department Of Advanced Materials Science Graduate School Of Frontier Sciences University Of Tokyo:cr

• Okamoto Hiroshi

  Department Of Advanced Biological Sciences For Regeneration (kotobiken Medical Laboratories) Tohoku

• Yamashita Masahiro

  Department Of Chemistry Graduate School Of Science Tohoku University

• Yamashita Masahiro

  Department Of Chemistry Graduate School Of Science Tohoku University And Crest Japan Science And Tec

• Yamashita Masahiro

  Department Of Chemistry Faculty Of Science Tokyo Metropolitan University

• Okamoto Hiroshi

  Correlated Electron Research Center (cerc) National Institute Of Advanced Industrial Science And Tec

• Okamoto Hiroshi

  Institute for Materials Research, Tohoku University

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