Ultrafast Phase Control in One-Dimensional Correlated Electron Systems(<Special Topics>Photo-Induced Phase Transitions and their Dynamics)
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概要
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One-dimensional (1D) correlated electron systems are good targets for the exploration of photoinduced phase transitions (PIPTs). This is because photocarrier generations and/or charge transfer (CT) excitations by lights can stimulate instabilities inherent to the 1D nature of electronic states through strong electron-electron interactions and electron (spin)-lattice interactions. In this paper, we review the ultrafast dynamics of three typical PIPTs observed in 1D correlated electron systems : 1) a photoinduced transition from a Mott insulator to a metal in a halogen-bridged Ni-chain compound, [Ni(chxn)_2Br]Br_2 (chxn=cyclohexanediamine); 2) a photoinduced melting of a spin-Peierls phase in an organic CT compound, K-tetracyanoquinodimethane (TCNQ); 3) a photoinduced transition between neutral (N) and ionic (I) states in an organic CT compound, tetrathiafulvalene-p-chloranil (TTF-CA). The primary dynamics of these PIPTs are discussed on the basis of the results of femtosecond pump-probe spectroscopy.
- 社団法人日本物理学会の論文
- 2006-01-15
著者
-
Okamoto Hiroshi
Department Of Cardiovascular Medicine Hokkaido University Hospital
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Iwai Shinichiro
Department Of Physics Faculty Of Science Tohoku University:nanostructure And Material Property Group
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