Structural Studies on Superionic Glass AgI-Ag_2O-MoO_3

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概要

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• Superionic conducting glass of the mole percent 60% Ag I-20% Ag. O-20% Mob.was prepared by rapid quenching from the melt. EXAFS and X-ray RDF studies indicate the presence of strong Ag-I interactions with r...=2.S7 A. Two Ag-0 interaclions whose distances differ by 0.38 A are also indicated. X-Ray RDF studies alsoyield r,. .=2. 1 A and the coordination number of oxygen around Mo, n..-.=5.7. Amodel is proposed which consists of a three dimensional network of distorted Mob.octahedra, which are 6, 4, and 2-corner shared leading to large channels in the structure. The Ag" tons form bonds and secondary interactions with both non-bridgingand bridging oxygen atoms in the network. The I tons surround the Ag" tons in thevoids created by the glass network. The results show that Ag" and I tons are highlydispersed in the glass network and cluster formation was not found as proposed byearlier workers.

• 社団法人日本物理学会の論文
• 1990-04-15

著者

• Nomura Masao

  Institute Of Physics College Of Arts And Sciences University Of Tokyo

• OHTAKI Hitoshi

  Coordination Chemistry Laboratories, Institute for Molecular Science

• Yamaguchi Tomohiko

  Department Of Chemical Systems National Institute Of Materials And Chemical Research (nimc)

• YAMAGUCHI Toshio

  Department of Physics, Tokyo Women's Medical University

• Nomura Mitsuhiro

  Institute Of Physics University Of Tsukuba:(present Address)fuji Electric Co. Ltd.

• Tsuyoshi Yamaguchi

  Faculty Of Engineering Shizuoka University

• Ohtaki H

  Coordination Chemistry Laboratories Institute For Molecular Science

• Ohtaki Hitoshi

  Coordination Chemistry Laboratories Institute For Molecular Science

• Nomura Masaharu

  Photon Factory High Energy Accelerator Research Organization (kek)

• Seshasayee M.

  Department of Physics, Indian Institute of Technology

• Seshasayee M.

  Department Of Physics Indian Institute Of Technology

• Yamaguchi Toshio

  Department Of Chemistry Faculty Of Science Fukuoka University

• Rajalakshmi A.

  Department of Physics,Indian Institute fo Technology,Madras,India

• Yamaguchi Toshio

  Department of Chemical Engineering, Tokyo University of Agriculture and Technology

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