A Structural Study on AgI-Ag_2O-CrO_3 Glass

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概要

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• A structural investigation for a 50AgI-20Ag_2O-30CrO_3 (in mole %) glass has been carried out by using X-ray diffraction (XRD) and the extended X-ray absorption fine structure (EXAFS) techniques. The analysis of the EXAFS spectrum of the glass at the Ag K-edge reveals that the distance between a silver (I) and an iodide ions, r_<Ag-I>, and the average number of iodide ions around an Ag^+, n_<Ag-I>, are 2.874(4)Å and 1.6(1), respectively. Two Ag-O distances separated by only 0.38 Å (Δr_<Ag-I>) are deconvoluted from the total Ag-O peak in the spectrum. The results by the X-ray diffraction measurement coincide with those by the EXAFS study within experimental uncertainties : r_<Ag-I>=2.860(1)Å, n_<Ag-I>=1.34(1), and Δr_<Ag-I>=0.35Å. The intramolecular structural parameters of CrO_3 are determined to be r_<Cr-O>=1.718 Å, and n_<Cr-O>=5.58. Short range ordering of atoms is discussed on the basis of the radial distribution function (RDF).

• 社団法人日本物理学会の論文
• 1993-02-15

著者

• Nomura Masao

  Institute Of Physics College Of Arts And Sciences University Of Tokyo

• OHTAKI Hitoshi

  Coordination Chemistry Laboratories, Institute for Molecular Science

• NOMURA Masaharu

  Photon Factory, Institute of Materials Structure Science, KEK

• Yamaguchi Tomohiko

  Department Of Chemical Systems National Institute Of Materials And Chemical Research (nimc)

• YAMAGUCHI Toshio

  Department of Physics, Tokyo Women's Medical University

• Nomura Mitsuhiro

  Institute Of Physics University Of Tsukuba:(present Address)fuji Electric Co. Ltd.

• Tsuyoshi Yamaguchi

  Faculty Of Engineering Shizuoka University

• Patnaik S.

  Department of Botany, Khallikote College

• Patnaik S.

  Department Of Botany Khallikote College

• Patnaik S.

  Department Of Physics Indian Institute Of Technology

• Ohtaki H

  Coordination Chemistry Laboratories Institute For Molecular Science

• Ohtaki Hitoshi

  Coordination Chemistry Laboratories Institute For Molecular Science

• Nomura Masaharu

  Photon Factory High Energy Accelerator Research Organization (kek)

• Seshasayee M.

  Department of Physics, Indian Institute of Technology

• Seshasayee M.

  Department Of Physics Indian Institute Of Technology

• Yamaguchi Toshihisa

  Department Of Applied Physics Chubu Institute Of Technology

• Yamaguchi Toshio

  Department Of Chemistry Faculty Of Science Fukuoka University

• Yamaguchi Toshio

  Department of Chemical Engineering, Tokyo University of Agriculture and Technology

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