Mechanism of Superconductivity in Quasi-Two-Dimensional Organic Conductor β-(BDA-TTP) Salts(Condensed matter: electronic structure and electrical, magnetic, and optical properties)

概要

論文の詳細を見る
We investigate theoretically the superconductivity of two-dimensional organic conductors, β-(BDA-TTP)_2SbF_6 and β-(BDA-TTP)_2AsF_6, to understand the role of the spin and charge fluctuations. The transition temperature is estimated by applying random phase approximation to an extended Hubbard model wherein realistic transfer energies are estimated by extended Huckel calculation. We find a gapless superconducting state with a d_<xy>-like symmetry, which is consistent with the experimental results obtained by specific heat and scanning tunneling microscope. In the present model with an effectively half-filled triangular lattice, spin fluctuation competes with charge fluctuation as a mechanism of pairing interaction since both fluctuations have the same characteristic momentum q=(π, 0) for V being smaller than U. This is in contrast to a model with a quarter-filled square lattice, wherein both fluctuations contribute cooperatively to pairing interaction due to fluctuations having different characteristic momenta. The resultant difference in the superconductivity of these two materials is also discussed.
社団法人日本物理学会の論文
2008-09-15