Optical and magnetic properties of (DBTTF)2(Cu2Cl6) and (DBTTF)2(Cu2Br6) complexes.
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Optical reflection and magnetic susceptibility measurements of (DBTTF)<SUB>2</SUB>(Cu<SUB>2</SUB>Cl<SUB>6</SUB>) and (DBTTF)<SUB>2</SUB>(Cu<SUB>2</SUB>Br<SUB>6</SUB>) complexes were carried out. The analysis of the reflection spectra of the single crystals of these complexes shows that the electronic structure of DBTTF<SUP>+</SUP> cation molecules is typical of the dimer type configuration. The magnetic susceptibilities of these complexes were measured over a temperature range of 2–300 K. The magnetic behavior conforms to a modified Bleaney-Bowers equation, indicating the existence of the spin coupling within the Cu<SUB>2</SUB>Cl<SUB>6</SUB><SUP>2−</SUP> or Cu<SUB>2</SUB>Br<SUB>6</SUB><SUP>2−</SUP> dimers and the antiferromagnetic spin interaction between Cu<SUB>2</SUB>Br<SUB>6</SUB><SUP>2−</SUP> dimers.
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