Photochemistry of host-guest complex. III. Effect of guest cation on the photoreactivity of acetophenone oxime derivatives having crown ether moiety.
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概要
- 論文の詳細を見る
The <I>syn-anti</I> isomerization of acetylbenzocrown ether oximes was stimulated by the complex-formation with sodium ion. The photolysis of these oximes gave mother ketones and amides through an oxaziridine intermediate. The photolysis of the oximes was depressed by the formation of host-guest complexes. Reactivity in the photolysis of the crown ether oximes corresponds to that of 3,4-dimethoxyacetophenone oxime, whereas the reactivity of the complexed crown ether oxime with sodium ion corresponds to that of <I>p</I>-cyanoacetophenone oxime. Such behavior is explained by the change of the electronic properties of excited states of acetophenone oxime chromophore, which enhances the intersystem crossing.
- 公益社団法人 日本化学会の論文
著者
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Suzuki Atsushi
Department Of Animal Husbandry Faculty Of Agriculture Tohoku University
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Tada Masaru
Department Of Chemistry School Of Science And Engineering Waseda University
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Hirano Hideki
Department of Chemistry, School of Science and Engineering, Waseda University
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