Absorption and fluorescence spectra of anthracenecarboxylic acids. II. 1- and 2-anthroic acids.
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概要
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The absorption and fluorescence spectra of 1- and 2-anthroic acids (1- and 2-anthracenecarboxylic acids) in alcoholic solvents have been observed as a function of solute concentration. It was revealed that 1- and 2-anthroic acids form hydrogen-bonded dimers in their ground states. The equilibrium constants for dimer formation are : 1.2×10<SUP>4</SUP> mol<SUP>−1</SUP>1 for 1-anthroic acid in methanol and 2.0×10<SUP>4</SUP> mol<SUP>−1</SUP>1 for 2-anthroic acid in ethanol. Owing to dimer formation, the lowest frequency absorption band of 1-anthroic acid was uniformly displaced to the red, while that of 2-anthroic acid was distinctly resolved into two bands. The band assignment was confirmed by the method of photoselection. No excimer-type fluorescence was observed in 1- and 2-anthroic acids. The lack of mirror-symmetry relationship between the absorption and fluorescence spectra of 1-anthroic acid is explained by the geometrical relaxation in its excited state.
- 公益社団法人 日本化学会の論文
著者
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Fujii Tsuneo
Department Of Chemistry And Materials Engineering Faculty Of Engineering Shinshu University
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Suzuki Satoshi
Department Of Advanced Cardiac Therapeutics Fukushima Medical University
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Yamanaka Shigeru
Department of Chemistry, Faculty of Science, Okayama University of Science
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Yamanaka Shigeru
Department of Industrial Chemistry, Faculty of Engineering, Shinshu University
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Yoshiike Nobuyuki
Department of Industrial Chemistry, Faculty of Engineering, Shinshu University
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Hayashi Zenro
Department of Industrial Chemistry, Faculty of Engineering, Shinshu University
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Fujii Tsuneo
Department of Chemistry and Material Engineering, Faculty of Engineering, Shinshu University
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