Electron Spin Resonance Study of TMCC : Mn^<2+>
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概要
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Electron spin resonance study of Mn" ions doped in (CH.).NCdC]3 (TMCC)is made at K-band frequency from room temperature to liquid nitrogen tempera-ture. ESR spectrtunn of uniaxial symmetry is obtained at room temperature. Thesrectrum channes to a rhombic one at 7'.z=]]2.4fO.1 K corresponding tohexagonal-to-monoclinic transition of the host crystal. The spectrum patternchanges at T..=96.0f0.] K correspondjng to the second transitjon which has notbeen reported earlier. Tlae nunaber of inequivalent Mn" sites becomes twowhereas there is one Mn" site above T... Temperature variation of hyperfineinteraction constant A and crystal field parameters D and E are presented. Relationbetween ESR spectrum pattern and crystal symntetry is discussed.
- 1977-05-15
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