Theoretical Study of X-Ray Photoemission, X-Ray Absorption and Resonant X-Ray Emission Spectroscopy at MnL_<2,3> Edge of Mn Films on Ag (Condensed Matter : Electronic Structure, Electrical, Magnetic and Optical Properties)
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概要
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Extending a previous study [Phys. Rev. B 68 (2003) 035407], we present calculations for the core-level X-ray photoemission (XPS), X-ray absorption (XAS) and resonant X-ray emission spectra (RXES) at MnL_<2,3> edge in Mn thin films on Ag (001) and related structures, namely an adsorbed Mn monolayer (ML) on Ag (001) [i. e. Mn/Ag (001)], a "buried" one [i. e. Ag/Mn/Ag (001)], an adsorbed bilayer Mn/Mn/Ag (001), a free standing Mn ML, bulk body-centered-tetragonal (bet) Mn, a Mn impurity in Ag, and a single Mn atom on Ag (001). Very good agreement with experiment is obtained in 2p XPS. Using the same parameter values, we could also reproduce the experimental 2pXAS spectra of the Mn/Ag (001) system. The calculated RXES spectra present satellite structures which are very sensitive to the hybridization strength. We have also studied the dependence of the different spectra on the effective Coulomb parameter U_<dd>. The XAS and RXES spectra show a strong dependence on U_<dd>, which allows to estimate its value.
- 社団法人日本物理学会の論文
- 2004-05-15
著者
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TAGUCHI Munetaka
RIKEN/SPring-8
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Taguchi Munetaka
Riken
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KOTANI Akio
Institute for Solid State Physics,University of Tokyo
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Parlebas Jean-claude
European Synchrotron Radiation Facility:(present Address) Laboratoire De Recherches Fur La Reactivit
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KRUGER Peter
SPring-8
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Kotani Akio
Institute For Solid State Physics The University Of Tokyo
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Kotani Akio
Institut De Physique Et Chimiedes Materiaux De Strasbourg Cnrs
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