A Simplified Theory of Liquid-Solid Transitions. III : Hard-Core Transitions
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概要
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The hard-sphere transition predicted by computer experiments is theoretically studied with the aid of the expandable-lattice theory of liquid-solid transitions developed in previous two papers. The freezing and melting points are thus given in the mean energy approximation by P/kT_<ρc>=2.3577, ρf/ρc=0.6819, ρm/c=0.9053, where ρc is the closest-packed density √<2>/ro^3, ro being the core diameter. Characteristic features of the hard-sphere transition are clarified in comparison with fluid-solid transitions in the systems of molecules interacting with the soft-core potentials (ro/r)^n, (12≦n<∞). Thus a unifying viewpoint is obtained for treating phase transitions in the Len-nard-Jones, soft-core and hard-core systems.
- 理論物理学刊行会の論文
- 1972-11-25
著者
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OKAMOTO Hisao
Department of Information Science, Kochi University
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Mori Hazime
Department Of Applied Physics Faculty Of Engineering Kyushu University
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Isa Shiro
Department Of Physics Kyushu University
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Isa Shiro
Department Of Physics Faculty Of Science Kyushu University
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Furukawa Hiroshi
Department Of Cardiology Okayama Central Hospital
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Furukawa Hiroshi
Department Of Applied Chemistry Faculty Of Engineering Nagasaki University
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