High-Field Magnetism of the Spin-Ladder Material Na2Fe2(C2O4)3(H2O)2
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概要
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We report the results of our magnetic susceptibility, magnetization, and multi-frequency electron spin resonance (ESR) measurements on single crystals of the two-leg spin-ladder material Na2Fe2(C2O4)3(H2O)2. Magnetization processes in magnetic fields up 53 T at 1.3 K paralell ($H\parallel a$) and perpendicular ($H\perp a$) to the leg direction show a gradual increase compared with those of the isomorphous compound Na2Co2(C2O4)3(H2O)2, which was well explained by an isolated antiferromagnetic dimer model. Thus, we calculated the magnetic susceptibilities and magnetizations on the basis of a two-leg ladder model with a fictitious spin ($S$) one by a quantum Monte Carlo method and a density-matrix renormalization group method, respectively. These calculated results, however, did not agree well with the experimental ones. Therefore, we regarded Na2Fe2(C2O4)3(H2O)2 as an isolated $S = 1$ antiferromagnetic dimer with not only the anisotropy of the exchange interactions due to the truncation of spin space but also single-ion anisotropy. Consequently, we obtained good agreement between the experimental and calculated results on the magnetic susceptibilities, magnetizations, ESR resonance modes, and specific heat.
- 2009-12-15
著者
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Todo Synge
Department Of Applied Physics University Of Tokyo:crest Japan Science And Technology Agency
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Honda Zentaro
Faculty Of Engineering Saitama University
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Hagiwara Masayuki
Kyokugen (center For Quantum Science And Technology Under Extreme Conditions) Osaka University
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Yamaguchi Hironori
Kyokugen (center For Quantum Science And Technology Under Extreme Conditions) Osaka University
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Kimura Shojiro
Kyokugen (center For Quantum Science And Technology Under Extreme Conditions) Osaka University
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Kindo Koichi
ISSP, The University of Tokyo, 5-1-5 Kashiwanoha, Kashiwa, Chiba 277-8581
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OKUNISHI Kouichi
Department of Applied Physics, Graduate School of Engineering Osaka University
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Okunishi Kouichi
Department of Physics, Niigata University, Niigata 950-2181
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Yamaguchi Hironori
KYOKUGEN, Osaka University, Toyonaka, Osaka 560-8531
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Kimura Shojiro
KYOKUGEN, Osaka University, Toyonaka, Osaka 560-8531
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Todo Synge
Department of Applied Physics, University of Tokyo, Bunkyo, Tokyo 113-8656
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