Thermoelectric Properties of Rare Earth-doped SrTiO3 Using Combination of Combustion Synthesis (CS) and Spark Plasma Sintering (SPS)
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概要
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Thermoelectric properties of combustion synthesized and spark plasma sintered rare-earth-doped (La, Sm, Gd, Dy and Y) SrTiO3 was investigated from room temperature to 870 K from viewpoint of energy and time saving without deterioration in thermoelectric properties. All single phases of rare-earth-doped SrTiO3 were successfully synthesized and sintered with high densities. With temperature increasing, the absolute value of Seebeck coefficient of all the samples increased and the electric conductivity decreased; the power factor of all the samples decreased except Y-doped sample in the considering temperature range. In all the samples, the La-doped sample and the Y-doped sample had the highest and lowest power factor, respectively. The figure of merit of La-doped samples with different doping amounts was evaluated and the maximum figure of merit 0.22 was obtained at 800 K from Sr0.92La0.08TiO3 sample. Comparing Y and La-doped samples prepared by our synthesis method with that of conventional solid-state reaction method, the thermoelectric properties of our samples were relatively higher. Thus the combination of combustion synthesis and spark plasma sintering has a potential to prepare perovskite-oxide materials with relatively higher thermoelectric properties for high-temperature application.
- 社団法人 日本鉄鋼協会の論文
著者
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Akiyama Tomohiro
Center for Advanced Research of Energy Conversion Materials, Hokkaido University
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Okinaka Noriyuki
Center for Advanced Research of Energy and Materials, Hokkaido University
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ZHANG Lihua
UBST
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Zhang Lihua
University of Science and Technology Beijing
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