Isotope Ratio Measurement of Uranium in Safeguards Environmental Samples by Inductively-Coupled Plasma Mass Spectrometry (ICP-MS)
スポンサーリンク
概要
- 論文の詳細を見る
In order to measure isotope ratio of uranium in safeguards environmental samples with ICP-MS precisely, production of polyatomic ions of IrAr, PtAr and AuAr was measured and mass bias of ICP-MS is investigated by using isotopic standards of uranium and lead. The intensities of IrAr, PtAr and AuAr relative to the atomic ions were found to be 1.8×10−6, 1.6×10−5 and 4.1×10−5, respectively. The production of 193Ir40Ar is too small to interfere with the measurement of 233U, if the concentration of Ir is the same level as that of 233U. However, there is possibility that the presence of Pt and Au interferes with the measurement of minor isotopes of uranium and 237Np. On the other hand, the mass biases of 235U/238U and 208Pb/206Pb were measured with the parameter of 238U16O/238U. Since unexpected change of the mass bias during measurements causes frequently erroneous results, the monitoring of 238U16O/238U is effective for the precise isotope ratio measurement.
- 社団法人 日本原子力学会の論文
- 2002-04-25
著者
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WATANABE Kazuo
Department of Pathology, Fukushima Medical University Hospital
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SHIMOTAKAHARA Sakurako
School of Pharmacy, Tokyo University of Pharmacy and Life Science
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ESAKA Fumitaka
Department of Applied Chemistry, Faculty of Science, Science University of Tokyo
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TAKAHASHI Masato
Department of Fine Materials Engineering,Faculty of Textile Science and Technology,Shinshu Universit
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Esaka Fumitaka
Nuclear Science And Engineering Directorate Japan Atomic Energy Agency
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Esaka Fumitaka
Department Of Applied Chemistry Faculty Of Science Science University Of Tokyo
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Sakurai Satoshi
Nuclear Science And Engineering Directorate Japan Atomic Energy Agency (jaea)
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Magara Masaaki
Nuclear Science And Engineering Directorate Japan Atomic Energy Agency
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Usuda S
Nuclear Science And Engineering Directorate Japan Atomic Energy Agency
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WATANABE Kazuo
Japan Atomic Energy Agency
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Hanzawa Yukiko
Department Of Environmental Sciences Japan Atomic Energy Research Institute
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MAGARA Masaaki
Department of Environmental Sciences, Japan Atomic Energy Research Institute
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SAKAKIBARA Takaaki
Department of Environmental Sciences, Japan Atomic Energy Research Institute
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KUROSAWA Setsumi
Department of Environmental Sciences, Japan Atomic Energy Research Institute
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SAKURAI Satoshi
Department of Environmental Sciences, Japan Atomic Energy Research Institute
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USUDA Shigekazu
Department of Environmental Sciences, Japan Atomic Energy Research Institute
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Watanabe Kazuo
Department Of Pathology Fukushima Medical University Hospital
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Kurosawa Setsumi
Department Of Environmental Sciences Japan Atomic Energy Research Institute
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Sakakibara Takaaki
Department Of Environmental Sciences Japan Atomic Energy Research Institute
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Takahashi Masato
Department Of Environmental Sciences Japan Atomic Energy Research Institute
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Watanabe K
Japan Atomic Energy Research Institute
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Watanabe Kazuo
Department Of Biology School Of Science Nagoya University
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Watanabe Kazuo
Department Of Biology Faculty Of Science Osaka University
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WATANABE Kazuo
Research Group for Analytical Science, Division of Environment and Radiation Sciences, Japan Atomic Energy Agency
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