A theoretical approach to the dielectric relaxation of alcohol solutions.
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概要
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The dielectric relaxation mechanism of primary alcohols in solutions of various solvents with and without a hydrogen-bonding capacity was theoretically studied using the concept of the chemical equilibrium between hydrogen-bonded chain multimers and that between the multimers and solvents. The dipole-inversion processes originating from the successive rotation of the hydroxyl groups of the hydrogen-bonded multimers were considered to play the dominant role in the dielectric relaxation of alcohol solutions. By applying the one-dimensional random-walk process to the dipole inversion, we estimated the effect of dilution upon the dielectric relaxation times of primary alcohol in solution. The results of our calculation appear to explain the experimental data.
著者
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Minami Ryuichi
Department Of Chemistry School Of Science And Engineering Waseda University:(present Address) Depart
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Sato Hiroshi
Department Of Anatomy And Developmental Neurobiology Institute Of Health Biosciences The University
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Takahashi Hiroaki
Department Of Biochemistry And Molecular Biology Graduate School Of Science And Engineering Saitama
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Itoh Koichi
Department of Applied Chemistry, Graduate School of Engineering, Nagoya University
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Higasi Keniti
Department of Chemistry, School of Science and Engineering, Waseda University
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