General Theory of Decay Processes in Molecules : A Green Function Treatment
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概要
- 論文の詳細を見る
In this paper a unified treatment of the decay theory is presented to reformulate the existing one in a more explicit form by treating radiative and vibronic interactions simultaneously. This treatment is based upon the Green function formulation in terms of the second quantization. Here the molecular eigenstate is treated as a Fermion. The retarded. Green function related to any physical processes is obtained by use of the method of equation of motion. From the analy sis of the self-energy part, one and two-photon processes are discussed in detail. First, in order to compare the present treatment with perturbation theory or the configuration interaction method, it is applied to a simple system. Next, an application to a three-level system shows a good agreement with the results of Mower's theory. Finally, for the system consisting of a discrete state and a continuum, the radiative decay in the case of internal conversion is properly discussed under the approximation that only the diagonal part of the self-energy part is taken into account.
- 理論物理学刊行会の論文
- 1973-08-25
著者
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Nishikawa Kiyoshi
Department Of Electrical Engineering Tokyo Metropolitan University
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Aono Shigeyuki
Department Of Chemistry College Of Arts And Sciences Chiba University
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Nishikawa Kiyoshi
Department Of Chemistry Faculty Of Science Kanazawa University
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AONO Shigeyuki
Department of Chemistry, Faculty of Science Kanazawa University
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NISHIKAWA Kiyoshi
Department of Chemistry, Faculty of Science Kanazawa University
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