Charge-Transfer Satellite in Ce@C82 Probed by Resonant X-ray Emission Spectroscopy
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概要
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The electronic structure of metallofullerene Ce@C82 is probed by resonant x-ray emission spectroscopy at the Ce L_{3} absorption edge. We observed a satellite structure in x-ray absorption and resonant emission spectra for Ce@C82, which, we show, corresponds to the charge transfer induced by the core--hole potential in the final state, similarly to Pr@C82. This charge-transfer satellite may be a common feature in metallofullerenes. The temperature dependence of the electronic structure is also investigated.
- 2011-01-15
著者
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YAMAOKA Hitoshi
Harima Institute, RIKEN (The Institute of Physical and Chemical Research)
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Ito Yoshiaki
Institute For Chemical Research Kyoto University
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KUBOZONO Yoshihiro
Faculty of Science, Okayama University
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Oohashi Hirofumi
Harima Office National Institute For Materials Science
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Tochio Tatsuki
Department Of Physics Faculty Of Science Kobe University
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Tochio Tatsuki
Department of Physics, Kobe University, Kobe 657-8501, Japan
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Kotani Akio
Harima Institute, RIKEN (The Institute of Physical and Chemical Research), Sayo, Hyogo 679-5148, Japan
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Yamaoka Hitoshi
Harima Institute, RIKEN (The Institute of Physical and Chemical Research), Sayo, Hyogo 679-5148, Japan
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Vlaicu Aurel
National Institute of Material Physics, Bucharest-Magurele 077125, Romania
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Yoshikawa Hideki
Harima Office, National Institute for Materials Science, Sayo, Hyogo 679-5148, Japan
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Kubozono Yoshihiro
Faculty of Science, Okayama University, Okayama 700-8530, Japan
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Yoshikawa Hideki
Harima Office (SPring-8 BL15XU), National Institute for Materials Science, Mikazuki, Hyogo 679-5198, Japan
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