Production of hydrogen by photochemical splitting of water using diammonium tetrathiomolybdate as photocatalyst.
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概要
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Hydrogen gas is generated at the cathode when the anode compartment of a photogalvanic cell anode/(NH<SUB>4</SUB>)<SUB>2</SUB>MoS<SUB>4</SUB>(aq, satd.)//5M HCl (aq)/cathode is illuminated. The photocurrent generated rises slowly with time and reaches a limiting value. A mechanism is suggested involving the conversion of Mo(VI) to Mo(V) and the formation of OH radicals, as evidenced by development of paramagnetism on irradiation. Although the photocatalyst is susceptible to hydrolysis, it can be easily regenerated by passing H<SUB>2</SUB>S.
- 公益社団法人 日本化学会の論文
著者
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Chatterjee A.
Department Of Chemistry University College Of Science
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Das K.
Department Of Applied Geology Ism University
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Bhattacharya A.
Department Of Medicine University Of Texas Health Science Center At San Antonio
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Rohatgi-Mukherjee K.
Department of Chemistry, Jadavpur University
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Chatterjee A.
Department of Chemistry, Jadavpur University
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Bhattacharyya R.
Department of Chemistry, Jadavpur University
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Basu J.
Department of Chemistry, Jadavpur University
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Bhattacharya A.
Department of Chemistry, Jadavpur University
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Das K.
Department of Chemistry, Jadavpur University
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