Radiation treatment of exhaust gases. VII. NO decomposition in NO-N2 and NO-rare gas mixtures.:NO Decomposition in NO-N<SUB>2</SUB> and NO-Rare Gas Mixtures
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概要
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The NO decomposition by electron beam irradiation was studied in the NO-N<SUB>2</SUB> and NO-rare gas mixtures. The NO decomposition yields, G(-NO), at low doses in the case of the 500 ppm NO initial concentration were 4.0, 4.4 and 1.2 for the NO-N<SUB>2</SUB>, NO-He and NO-Ar mixtures respectively. A small amount of NO<SUB>2</SUB> was formed by irradiation of these mixtures. The NO decomposition is mainly attributable to the attacks of N and N<SUB>4</SUB><SUP>+</SUP> (or N<SUB>2</SUB><SUP>+</SUP>), formed by the radiolysis of N<SUB>2</SUB>, on NO in the NO-N<SUB>2</SUB> mixture, and to the attacks of R<SUP>+</SUP> and R*, formed by the radiolysis of a rare gas (R), on NO in the NO-rare gas mixture. The NO decomposition in the NO-N<SUB>2</SUB> mixture was depressed markedly by the addition of a small amount of O<SUB>2</SUB>. This may be mainly attributable to scavenging of N and N<SUB>4</SUB><SUP>+</SUP> (or N<SUB>2</SUB><SUP>+</SUP>) by O<SUB>2</SUB>2.
- 一般社団法人 日本原子力学会の論文
著者
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Suzuki Nobutake
Takasaki Radiation Chemistry Research Establishment Japan Atomic Energy Research Institute
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Nishimura Koichi
Takasaki Radiation Chemistry Research Establishment Japan Atomic Energy Research Institute
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WASHINO Masamitsu
Takasaki Radiation Chemistry Research Establishment, Japan Atomic Energy Research Institute
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TOKUNAGA Okihiro
Takasaki Radiation Chemistry Research Establishment, Japan Atomic Energy Research Institute
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