Radiation treatment of exhaust gases. IX. Analysis of NO and NO2 decomposition in NO-N2 and NO2-N2 mixtures by computer simulation.:Analysis of NO and NO<SUB>2</SUB> Decomposition in NO-N<SUB>2</SUB> and NO<SUB>2</SUB>-N<SUB>2</SUB> Mixtures by Computer S
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概要
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The computer simulation method has been applied to the analysis of the NO and NO<SUB>2</SUB> decomposition in the NO-N<SUB>2</SUB> and NO<SUB>2</SUB>-N<SUB>2</SUB> mixtures by electron beam irradiation. The calculated results regarding the NO and NO<SUB>2</SUB> decomposition were in good agreement with the experimental results in both mixtures. The NO and NO<SUB>2</SUB> decomposition is mainly induced by the radical reactions and is hardly induced by the ion reactions. That is, the NO decomposition in the NO-N<SUB>2</SUB> mixture is mainly induced by the attack of N formed by the radiolysis of N<SUB>2</SUB>. The NO<SUB>2</SUB> decomposition in the NO<SUB>2</SUB>-N<SUB>2</SUB> mixture is induced not only by the attack of N, but also by the attack of 0 formed through the reaction of NO<SUB>2</SUB> with N at low doses. At high doses, the decomposition of NO formed through the reactions of NO<SUB>2</SUB> with N and with 0 is mainly induced by the attack of N, in contrast to the NO<SUB>2</SUB> decomposition by the attacks of N and O at low doses. The <I>G</I> value of the formation of N(<I>G</I> (N)) by the computer simulation was 2.0.
- 一般社団法人 日本原子力学会の論文
著者
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Suzuki Nobutake
Takasaki Radiation Chemistry Research Establishment Japan Atomic Energy Research Institute
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Nishimura Koichi
Takasaki Radiation Chemistry Research Establishment Japan Atomic Energy Research Institute
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WASHINO Masamitsu
Takasaki Radiation Chemistry Research Establishment, Japan Atomic Energy Research Institute
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TOKUNAGA Okihiro
Takasaki Radiation Chemistry Research Establishment, Japan Atomic Energy Research Institute
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