Dipole Correlation Functions of Non-interacting Symmetric Vib-rotors
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概要
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Dipolar correlation functions of non-interacting symmetric top molecules were obtained by quantum mechanical calculation. The effect of the rotation-vibration interaction on the correlation function is discussed, taking the constant ζ of the Coriolis coupling and the asymmetry <I>I</I><SUB>x</SUB>/<I>I</I><SUB>z</SUB> as parameters. It is shown that the decay of the correlation function for perpendicular vibrations very much depends on the sign and the magnitude of ζ. Some relationships between the shape of the correlation function and the value of the parameters are given.
- 公益社団法人 日本化学会の論文
著者
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Shimizu Hiroshi
Faculty Of Environmental Information Keio University
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Yamashita Teruyo
Faculty of Pharmaceutical Sciences, Kyushu University
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