Molecular Orbitals and Third-Harmonic Generation for Symmetrically Substituted Benzylidene Aniline

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概要

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• Molecular orbitals and third-order susceptibility are calculated for terephthal-bis-(4-N, N-diethylamino aniline). The main mechanism of third-harmonic generation is explained approximately by a three-level system. The effect of the orbital shape upon the susceptibility is analyzed. It is found that molecular orbital distortion, due to introduced nitrogen atoms, enhances the transition moment between excited states, 1B_u-2A_g, and this contributes to the third-order susceptibility.

• 社団法人応用物理学会の論文
• 1992-03-15

著者

• Tomaru S

  Ntt Opto-electronics Laboratories Nippon Telegraph And Telephone Corporation

• Tomaru Satoru

  Ntt Opto-electronics Laboratories Nippon Telegraph And Telephone Corporation

• 神原 貴樹

  Chemical Resources Laboratory Tokyo Institute Of Technology

• KURIHARA Takashi

  NTT Opto-electronics Laboratories

• Kaino T

  Institute Of Multidisciplinary Research For Advanced Materials Tohoku University

• Kaino Toshikuni

  Ntt Opto-electronics Laboratories

• MORI Yuhei

  NTT Opto-electronics Laboratories, Nippon Telegraph and Telephone Corporation

• Mori Yuhei

  Ntt Opto-electronics Laboratories Nippon Telegraph And Telephone Corporation:(present Address) Davy-

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