ベンジル位アニオンの気相安定性に及ぼす置換基効果
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概要
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Relative gas phase stabilities of ring substituted benzylic anions were theoreticallydetermined using proton transfer equilibria.Substituent effects of these benzylic anions werecompared with one another to discuss what kind of electronic effects are important to determinethe gas phase stabilities. According to statistical analyses, saturation effect was found to beinfluential in addition to inductive and resonance effects. The third term shuold be added to theconventional Yukawa-Tsuno equation in order to correlate the stabilities of benzylic anions.
- 2009-03-31
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