Superconducting T′-La_<2-x>Ce_xCuO_4 Films Grown by Molecular Beam Epitaxy
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In this letter we report the synthesis of superconducting T′-La_<2-x>Ce_xCuO_4 on SrTiO_3(001)by molecular beam epitaxy. Although T′-La_<2-x>Ce_xCuO_4 with a very limited range of x can be prepared by bulk synthesis using rather complicated techniques, this compound is very easy to obtain by thin film synthesis. Crucial to our success was the use of SrTiO_3 substrates, which seems to stabilize the formation of the T′ structure by an epitaxial effect. The best T_c was 〜30K by onset and 〜28K by zero resistance, which was obtained for x=0.109. The resistivity showed a metallic temperature dependence, and the film's overall behavior was similar to that for the best(Nd, Ce)_2CuO_4 or(Pr, Ce)_2CuO_4 films. Moreover, the single phase of the T′ Structure formed for a composition range of 0.09<x<0.22, which is much wider than for previously reported bulk synthesis.
- 社団法人応用物理学会の論文
- 2000-06-01
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