Mossbauer Study of Supertransferred Hyperfine Field of ^<119>Sn (Sn^<4+>) in Ca_<1-x>Sr_xMnO_3
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概要
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Ca_<1-x>Sr_xMn_<0.99>Sn_<0.01>O_3(0≦x≦1) with (nearly) cubic perovskite structures were prepared and the magnetic hyperfine fields of ^<119>Sn(Sn^<4+>) were measured by the Mossbauer effect. The hyperfine fields arise from unpaired s electron spin densities transferred from Mn^<4+> ions (super-transferred hyperfine interaction). The hyperfine field for a tin ion was found to depend linearly upon the numbers of Ca^<2+> and Sr^<2+> ions in the neighboring divalent cation sites, with proportional coefficients having opposite signs. To explain experimental results two kinds of spin transfer processes contributing to the hyperfine field oppositely to each other have been considered, and spin transfer via a divalent cation is emphasized particularly. The hyperfine field at 0 K for Sn^<4+> in CaMnO_3 is -75 kOe, while +20 kOe for Sn^<4+> in SrMnO_3.
- 社団法人日本物理学会の論文
- 1975-09-15
著者
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SHINJO Teruya
Institute for Chemical Research,Kyoto University
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SHIMADA Masahiko
Institute of Multidisciplinary Research for Advanced Materials, Tohoku University
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TAKANO Mikio
Department of Physics, Toho University
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Takano Mikio
Department Of Chemistry Faculty Of Science Konan University
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TAKEDA Yasuo
Institute of Scientific and Industrial Research, Osaka University
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MATSUZAWA Takao
Institute for Chemical Research, Kyoto University
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Shimada Masahiko
Institute Of Multidisciplinary Research For Advanced Materials Tohoku University
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Matsuzawa Takao
Institute For Chemical Research Kyoto University
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Matsuzawa Takao
Institute For Chemical Research Kyoto University:(present Address) The Oarai Branch The Research Ins
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Shinjo Teruya
Institute For Chemical Research Kyoto Universiry
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Shimada M
Univ. Electro‐communications Tokyo
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Takeda Yasuo
Institute Of Scientific And Industrial Research Osaka University:(present Address) Synthetic Crystal
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Shimada Masahiko
Institute For Advanced Materials Processing Tohoku University
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Shimada Masahiko
Institute Of Scientific And Industrial Research Osaka University
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