Theoretical and Experimental Study of Resonant 3d X-Ray Photoemission and Resonant L_3M_<45>M_<45> Auger Transition of PdO : Condensed Matter: Electronic Properties, etc.

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概要

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• The observed 3d X-ray photoemission spectra (XPS), resonant 3dXPS (RXPS) at the L_3 edge and resonant L_3M_<45>M_<45> Auger electron spectra (RAES) of 4d transition metal oxide PdO are successfully analyzed by means of an impurity Anderson model. The importance of Pd 4d-O 2p hybridization effect is especially emphasized in the interpretation of observed spectra. It causes charge transfer satellites in 3dXPS and L_3M_<45>M_<45>RAES and mainly determined the structure of resonance enhancements in 3dRXPS. From the analysis of spectra, 4d-2p charge transfer energy Δ, 4d correlation energy U_<dd> and 4d-2p transfer integral pdσ are estimated to be 5.5eV, 4.5eV and 2.1eV, respectively. The character of the insulating energy gap of PdO is also theoretically investigated: PdO is classified as an intermediate-type insulator due to the strong 4d-2p hybridization.

• 社団法人日本物理学会の論文
• 2000-04-15

著者

• OKANE Tetsuo

  Department of Physics, Tohoku University

• Yoshii Kenji

  Department Of Cardiology Kurashiki Central Hospital

• Yoshii Kenji

  Department Of Synchrotron Radiation Research Japan Atomic Energy Research Institute

• UOZUMI Takayuki

  College of Engineering, Osaka Prefecture University

• Okane Tetsuo

  Department Of Synchrotron Radiation Research Japan Atomic Energy Research Institute

• Sasaki Teikichi

  Department Of Chemistry Japan Atomic Energy Research Institute

• Uozumi Takayuki

  College Of Engineering Osaka Prefecture University

• KOTANl Akio

  Institute for Solid State Physics, The University of Tokyo

• Kotanl Akio

  Institute For Solid State Physics The University Of Tokyo

• Sasaki T

  Department Of Synchrotron Radiation Research Japan Atomic Energy Research Institute

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