Optical Third Harmonic Generation by Molecular Vibration
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概要
- 論文の詳細を見る
A theoretical consideration of nearly resonant interaction between the infrared radiation and the anharmonic molecular vibration has been developed to evaluate an efficiency of third harmonic generation in the infrared by molecules. By suing the spectroscopecally measured molecular constants in the Morse function, the nonlinear susceptibilities for second and third harmonic generation are derived. The problem is treated both classically and quantum mechanically. It is found that the spectroscopic stability holds for the nonlinear susceptibility. Non-resonant interactions which usually occur in solids are also discussed briefly. A gas of molecules with random orientations cannot produce optical second harmonics. However, each molecule has the nonlinear susceptibility of second harmonic generation by its molecular vibration and it is found that the Miller's rule also holds for the molecular susceptibility.
- 社団法人日本物理学会の論文
- 1970-01-05
著者
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Shimoda Koichi
Department Of Physicas University Of Tokyo
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Ueda Yoshifumi
Department Of Pharmacology Gifu Pharmaceutical University
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Shimoda Koichi
Department Of Physics University Of Tokyo
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