Photoemission Study of Mixed-Valent Tm-monochalcogenides : Evidence of Electron-Correlation Effect in Different Tm-Core Levels (Condensed Matter: Electronic Structure, Electrical, Magnetic and Optical Properties)

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概要

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• Systematic results of the photoemission spectra for different core levels such as, Tm 4ρ, 5ρ and 3d in the mixed valent Tm-monochalcogenides (TmS, TmSe and TmTe) obtained by both experimentally and theoretically are reported. The effects of the electron-electron correlation due to the interaction between core-holes and 4f-electrons or the interaction between different configurations are considered to explain the spectral features, depending on the principal (n) and orbital quantum numbers of the core levels. Any sharp peak corresponding to a spin-orbital term is not observed especially from the n = 4 states. Instead, the multiplet structures are dominantly observed, and the physical identity of the spin-orbital peaks is totally or partially dissolved into the multiplets. Moreover, the electron-correlation effect is found to be dependent on the valence components (Tm^<2+> and Tm^<3+>). In the case of the Tm 4ρ core level, in which the principal quantum number is identical with the valence 4f, the correlation effect is stronger, and the configuration interaction is therefore considered to explain the spectral features. The photoemission spectra for the shallow core level Tm 5ρ also show the effect of electron correlation, but weaker than that for Tm 4ρ. This has been confirmed by the resonant photoemission spectroscopy taken at Tm 4d-4f absorption edges. In addition, the feature of Tm 3d photoemission spectra is discussed. All the experimental spectra are compared with the calculated ones. It is therefore understood that the electron correlation effect plays an important role on determining the various features in Tm 4ρ, 5ρ and 3d photoemission spectra.

• 社団法人日本物理学会の論文
• 2003-07-15

著者

• MATSUMURA Takeshi

  Department of Quantum Matter, ADSM, Hiroshima University

• KIMURA Shin-ichi

  UVSOR Facility, Institute for Molecular Science

• Shin-ichi Kimura

  Uvsor Facility Institute For Molecular Science

• SUZUKI Takashi

  Department of Biochemistry, University of Shizuoka, School of Pharmaceutical Sciences, Core Research

• Takagi S

  Department Of Quantum Matter Graduate School Of Advanced Sciences Of Matter Hiroshima University

• Tsutsui Satoshi

  Japan Synchrotron Radiation Research Institute Spring-8

• KOTANI Akio

  Institute for Solid State Physics,University of Tokyo

• 榊原 俊雄

  東大物性研

• 小谷 章雄

  SPring-8

• Tsutsui Satoshi

  Department Of Materials Science And Technology Iwate University

• 小谷 章雄

  理研 Spring-8:高エ研

• Matsumura T

  Adsm Hiroshima University

• Suzuki T

  Issp University Of Tokyo

• Nath Krishna

  Department Of Structural Molecular Science The Graduate University For Advanced Studies:(present Add

• Kimura S

  The Graduate School Of Science An Technology Kobe University

• Sasaki T

  Center For Geo-environmental Science Faculty Of Engineering And Resource Science Akita University

• Tatsuoka Sho

  Graduate School Of Science Tokyo Metropolitan University

• Suzuki N

  Riken (inst. Physical And Chemical Res.) Saitama

• Suzuki N

  Osaka Univ. Osaka Jpn

• Suzuki Naoshi

  Department Of Material Physics Osaka University

• Sugaya Takashi

  Issp University Of Tokyo

• Kimura S

  Graduate School Of Science And Technology Kobe University

• Kimura Shin-ichi

  Uvsor Facility Institute For Molecular Science

• Kimura Shin-ichi

  Division Of Mathematical And Material Science Graduate School Of Science And Technology

• OGASAWARA Haruhiko

  Institute for Solid State Physics, University of Tokyo

• Sakon Takuo

  Department Of Physics Faculty Of Science Tohoku University

• Kinoshita T

  Issp University Of Tokyo:spring-8 Jasri

• Kinoshita T

  Inst. Molecular Science Okazaki Jpn

• KINOSHITA Toyohiko

  UVSOR facility,Institute for Molecular Science

• Kotani Akio

  Department Of Mechanical Engineering Osaka University

• Haruyama Y

  Graduate School Of Science Laboratory Of Advanced Science And Technology For Industry (lasti) Univer

• Haruyama Yuichi

  Uvsor Facility Institute For Molecular Science:(present Address)laboratory Of Advanced Science And T

• Haruyama Yuichi

  Institute Of Physics University Of Tsukuba

• Ogasawara H

  Spring-8:(present Address)school Of Physics And Physics Research Division Seoul National Universty

• Ogasawara Haruhiko

  Institute For Solid State Physics University Of Tokyo

• Suzuki T

  Graduate School Of Science And Technology Chiba University

• Koizumi Tomohiro

  Faculty Of Technology Tokyo University Of Agriculture And Technology

• UFUKTEPE Yuksel

  UVSOR Facility, Institute for Molecular Science

• Tsutsui Satoshi

  Department Of Material Physics Faculty Of Engineering Science Osaka University

• Ufuktepe Yuksel

  Uvsor Facility Institute For Molecular Science

• Suzuki Taira

  Department Of Mterials Science And Technology Science University Of Tokyo

• 小谷 章雄

  理化学研究所播磨研究所

• Ogasawara Hiromitsu

  Department Of Materials Science And Technology Iwate University

• Kimura Shojiro

  Molecular Photoscience Research Center And Department Of Physics:(present Address)kyokugen Osaka Uni

• Kotani Akio

  Institute For Solid State Physics The University Of Tokyo

• Suzuki Takashi

  Department Of Biochemistry University Of Shizuoka School Of Pharmaceutical Sciences:core Research Fo

• Sasagawa Takao

  Graduate School Of Frontier Sciences University Of Tokyo

• Kinoshita Toyohiko

  Issp University Of Tokyo:spring-8 Jasri

• Matsumura Takeshi

  Department Of Physics Graduate School Of Science Tohoku University

• Matsumura Takeshi

  Department Of Cardiovascular Surgery Shin-tokyo Hospital

• Matsumura Takeshi

  Department Of Agrobiology And Bioresources Faculty Of Agriculture Hokkaido University

• Saito Takashi

  Institute For Chemical Research Kyoto University

• Kotani Akio

  Institut De Physique Et Chimiedes Materiaux De Strasbourg Cnrs

• Suzuki Takashi

  Department Of Anesthesia Showa University Northern Yokohama Hospital

• Suzuki Takashi

  Department Of Anatomic Pathology Tohoku University School Of Medicine

• KOTANI Akio

  Department of Physics, Tohoku University : Institute for Solid State Physics, University of Tokyo

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