Methematical Considerations in Chemical Kinetics of Radiation-Induced Polymerization
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概要
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The chemical kinetics of radiation-induced polymerization is mathematically investigated. The implication of the "stationary state" hypothesis, currently employed in kinetic treatments, is carefully examined. It is shown that the hypothesis is valid only in a certain time interval. Qualitative behaviors of the total number of polymer radicals as well as of polymer molecules as a function of time are derived without resorting to the stationary state hypothesis. In particular, the asymptotic behavior of the total number of radicals proves to be sensitive to the mode of termination reaction. It is also confirmed that the molecular size distribution approaches to the Poisson type asymptotically.
- 社団法人日本物理学会の論文
- 1961-05-05
著者
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Inokuti Mitio
Department Of Applied Physics Faculty Of Engineering
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Amemiya Ayao
Department Of Applied Mathematics Second Faculty Of Engineering And Department Of Dynamics First Fac
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Amemiya A.
Department of Applied Physics, Faculty of Engineering, The University of Tokyo
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Amemiya A.
Department of Applied Physics, Faculty of Engineering, University of Tokyo
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