The Effect of Electron Density and Electron Temperature on the Partial Oxidation of Benzene Using a Micro-Plasma Reactor

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概要

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• The effects of electron density and electron temperature on the partial oxidation of benzene using a micro-plasma reactor have been studied here. The plasma was generated by the dielectric barrier discharge at the atmospheric pressure. The electron density and electron temperature are key parameters for the plasma reaction of benzene. By changing the combinations of discharge conditions including the applied voltage, discharge gap, and discharge frequency, the electron density and electron temperature could be controlled. Applying the higher voltage, both the electron density and electron temperature were increased. Along with increasing the discharge frequency and reducing the discharge gap at a constant input power, the electron density increased whereas the electron temperature decreased. Higher electron densities and higher electron temperatures resulted in the enhancement of the benzene conversion. In addition, the phenol selectivity did not varied greatly with the change of electron density, while it was slightly enhanced with the increase of electron temperature. The micro-plasma reactor made it possible to change the electron density and electron temperature largely, and it has a potential to control chemical reactions effectively.

• 社団法人 化学工学会の論文
• 2007-09-01

著者

• Takaki Koichi

  Department Of Electrical And Electronic Engineering Iwate University

• SUZUKI Sho

  Department of Materials Engineering, School of Engineering, The University of Tokyo

• SEKIGUCHI Hidetoshi

  Department of Chemical Engineering, Tokyo Institute of Technology

• Sekiguchi Hidetoshi

  Dep. Of Chemical Engineering Tokyo Inst. Of Technol.

• Sekiguchi Hidetoshi

  Department Of Chemical Engineering Tokyo Institute Of Technology

• Suzuki Sho

  Dep. Of Chemical Engineering Tokyo Inst. Of Technol.

• Suzuki Sho

  Department Of Chemical Engineering Tokyo Institute Of Technology

• Suzuki Sho

  Department Of Chemical Engineering & Materials Science Doshisha University

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